Antonio M Garc í aGarc í a Cavendish Laboratory Cambridge University Pedro Ribeiro Lisbon Bermudez Cambridge C azalilla Tsinghua ID: 747518
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Slide1
Smaller is different and more: Low dimensional superconductivity for new physics and applications
Antonio M. García-García Cavendish Laboratory, Cambridge University
Pedro Ribeiro Lisbon
Bermudez
Cambridge
C
azalilla Tsinghua
MayohCambridge
Endo Paris, ENS
Paul
Chesler
Harvard
Tezuka
Kyoto
Hong Liu MIT
Lobos Maryland
Naidon
RIKENSlide2
Mavericks
MgB2 39K 2001 Akimitsu Cuprates ~100K 1986 Mueller & Bednorz
FeSC ~50K 2006 Hotsono
Quantum critical points ©
Superconductivity For Happiness
Trial and errorSlide3
LibrariansControl
Pb ~7K Al ~1K Sn ~3.7K Nb ~9.3K Thinner
Cleaner
Smaller
BCS + (weak) disorder, interactions..Thin films
Josephson Junctions
Nanowires
DFTSlide4
Enhancement of superconductivity? Mavericks meet Librarians
Theory does not driftExperimental ControlConventional SC in low dimensions Artificial
hetero,nano-
structures
Novel Interfaces FeSe
/STO, LAO/STO
True Design of Materials!
A revolution is going onSlide5
Abeles, Cohen, Cullen, Phys. Rev.
Lett., 17, 632 (1966) A.M. Goldman, Dynes, Tinkham…Thin Films?Crow, Parks, Douglass, Jensen,
Giaver, Zeller.... Slide6
Shape Resonances
Blatt, Thompson, Phys. Lett. 5, 6 (1963) Thin FilmsFluctuations?Charge neutrality?
Substrate?
>10Tc!
Bermudez, AGG, Phys. Rev. B 89, 064508 (2014) 89, 024510 (2014)
Yu, et al.,Rev
. B 14, 996 (1976)Slide7
A.M. Goldman et al.
PRL 62 2180 (1989)PRB 47 5931 (1993)
Smoother
Thinner
Disordered
Transition
BKT
(anti)Vortex unbindingSlide8
Xue et al., Science 306, 1915 (2004)
Shih et al., Science 324, 1314 (2009)2000 Atomic scale control
Pb
Size effects but not higher TcSlide9
STM
Epitaxial growthImpurities?
Xue
TsinghuaSlide10
LaAlO3
/SrTiO3 interfaceTriscone et al. , Nature 456 624 (2008)Control
Mannhart
et al., Nature 502, 528 (2013)
Tunability
Localization
Exotic Quantum Matter
TopologySlide11
Cuprates high Tc Heterostructures
Bozovic et al., Nature 455, 782 (2008) Higher Tc!! Slide12
Nature Comm. 3, 931 (2013),
Chinese Phys. Lett. 29 037402 (2012) Iron Based Heterostructures
Feng, et.
al, Nat. Commun. 5:5044 (2014)
Slide13
Bulk
FeSe8K!Slide14
STO is key!Slide15
Nano-grainsSlide16
Abeles, Cohen, Cullen, Phys. Rev.
Lett., 17, 632 (1966) A.M. Goldman, Dynes, Tinkham…Single grains?Crow, Parks, Douglass, Jensen,
Giaver, Zeller.... Slide17
Odd-even effects
~ Superconductivity? Isolated grain?Yes, superconductivity
1959
Ralph, Black,Tinkham, Superconductivity in Single
Metal Particles PRL 74, 3241-3244 (1995).
Rediscovery of
Richardson’s equationsNo yet quantitative Slide18
0 nm
7 nmSlide19
BCS superconductivity
Finite size effects
V
Δ
~
D
e-1/
V finite Δ=?
Shell Effects
Parmenter
, Phys. Rev. 166, 392 (1967)L ~ 5nm
Level Degeneracy
20T
c
!Slide20
>>
Heiselberg (2002): harmonic potentials, cold atomKresin, Ovchinnikov, Boyaci (2007) : Spherical, too high T
c
Peeters, et al, (2005-): BCS, BdG
in a wire, cylinder..
Olofsson
(2008): Estimation of fluctuations in BCS Devreese
(2006): Richardson equations in a boxGrainsSlide21
>>
Expansion in 1/kFL, /∆0
L ~ 10nm
AGG,
Altshuler, PRL 100, 187001 (2008) AGG,
Altshuler, PRB 83, 014510
(2011) Slide22
R ~ 4-30nm
Single, Isolated Sn and Pb grainsA gap is still observedTunneling conductance
Almost hemispherical
Kern
Bose
STM
0 nm
7 nmSlide23
+
Bose, AGG, Nature Materials 2010Slide24
Richardson’s equations
Static Path ApproachBrihuega, AGG, Ribeiro, Bose, Kern PRB 84,104525 (2011)Editor‘s SuggestionQuantum Fluctuations
Thermal Fluctuations
and
Beyond mean field
~ Slide25
Quantum + Thermal?Ribeiro and AGG, Phys.
Rev. Lett. 108, 097004 (2012)T, / Δ0 << 1 Divergences at intermediate T
Rossignoli and
CanosaAnn. of Phys. 275, 1, (1999)
Harmful Zero Modes
Polar coordinates
Quantum fluctuations ~ Charging effectsSlide26
Mason, et al, Nature Physics 8 59 (2012)
Josephson array? True phase coherence in single nanograins?
No
M
aybeSlide27
Engineering inhomogeneous materials
Nano-granularity Mayoh, AGG. PRB 90, 134513 (2014
)
James
Mayoh
Disorder,
Mayoh, AGG, 1412.0029 PRX (?)
Global
Tc > Bulk
T
c?
Topology, Matthews,
Ribeiro, and AGG, PRL 112, 247001(2014)
Inhomogeneous JJ arrays
Experimentally feasible
Charging effects
3D nano-spheres
Slide28
3D Array
H
O
M
O
G
E
NE
OUS
I
N
HO
MOGE
NEOU
SPercolation ?
T
#SCG
Schoen,
Zaikin
, Fazio
Charging
Hopping
Quasiparticles
1
N
ano-Grain
Tunnelling
+Slide29
Percolation?Tc
?T
#
SCgrains
Phase fluctuations?
R=5nm
=1nm =0.3Slide30
Packing = FCC, BCC, Cubic
Enhancement!
Patent
Mark
Blamire
CambridgeSlide31
SURPRISE!Slide32
Xue
Tsinghua
Lara BenfattoRome
Nano-granularity
Interface design
Xue
et.al PRB B91 060509(R) (2015)Engineering
FeSe/STOSlide33
Inhomogeneities by disorderCan disorder enhance superconductivity?
Global TcEnergy gapOrder parameter
Slide34
Some bad news
BdG too difficultBCS doable
b
ut valid only if
Slide35
Anderson TheoremMa & Lee 80’s
Localization and SC can coexist Trivedi et al., Meir 90’s Numerical BdG
Emergent granularity
Disorder and superconductivity
Gorkov, Anderson 50’s
(Do not worry about disorder)
Weak localization weakens SC
Maekawa, Finkelstein 80’s
Pseudogap, Goldstone, Higgs modes, gap distribution function
Sacepe
,
Benfatto,
RaychaudhuriMultifractal
disorderKravtsov
, MirlinSlide36
Enhancement of Tc by disorder
Bianconi, et al., Nature 466, 841 (2010)Fractal distributions of dopants
enhance Tc
in
cuprates
Inhomogeneities
Higher
T
c
PRL 108, 017002 (2012)
PRL, 98
, 027001 (2007)Slide37
Strong
multifractality
and superconductivity
~ 0.4
Feigelman
,
Ioffe
,
Kravtsov
,
Yuzbashyan
, Phys. Rev. Lett. 98, 027001 (2007)
I. S. Burmistrov, I. V.
Gornyi,
A. D. Mirlin, Phys. Rev. Lett. 108, 017002 (2012)
3d MITSlide38
Weak
multifractality and superconductivity
(Ultra) Thin films
2D + Spin orbit
1D + Long Range
energy dependence
J.
Mayoh
and AGG, PRB 92 174526 (2015)
Where?
What?
spatial distribution
Global
T
c
!
Can disorder enhance SC?
How?
Percolation
energy gap
Slide39
Still unrealistic
Why?
Inhomogenous
SC
Not true Tc
Slide40
Sacepe
et al., Nat. Phys. 7 239 (2011)
Global Tc?
Lemarie
,
Benfatto
, et al., PRB 87,
184509 (2013)
Tracy-
Widom?
Log-Normal distributionSlide41
Global Tc?
Enhancement?YesBut
Al is fine!
FeSe
/STO?
Slide42
Out of equilibrium superconductivitySlide43
Unbroken Phase
Broken phase Tc
T(t)
The out of equilibrium birth of a superfluid
Phys. Rev. X 5,
021015 (2015)
Hong Liu
MIT
Paul
Chesler
Harvard
Slide44
Kibble
J. Phys. A: Math. Gen. 9: 1387. (1976)Vortices in the sky
Causality
Generation of Structure
Cosmic strings
Weyler
, Nature 2008
Krusius
, 2006Slide45
t
Adiabatic
Adiabatic
Frozen
Kibble-
Zurek
mechanism
Zurek
Nature 317
(1985
) 505
T
cSlide46
KZ scaling with the quench speed
Too few defectsSlide47
Adiabatic at tfreeze?
Defects without a condensate?
is relevant
Chesler
, AGG, Liu
Issues with KZ
Too many defects
Phys. Rev. X 5,
021015 (2015)Slide48
ScalingLinear response
Slow Quenches
Frozen
Coarsening
Adiabatic
Frozen
Adiabatic
KZ
US
Slide49
t
eq is the relevant scaleNumericsU(1) theory with a gravity dualSlide50
Adiabatic
Non adiabatic
Slow quenchesSlide51
~
25 times less defects than KZ prediction!!Relevant for 4He, materials ?SlowFast
Slow
Fast
Slide52
Out of equilibriumQuantum InformationEmergent quantum matter
Thermalization, steady non-thermal, dynamical transitions Many-body Efimov in condensed matter, topology
Bounds on transport “Universal quantum constraints on the butterfly effect” D.
Berenstein, AGG, 1510.08870
Materials nano
-design
Interfaces
HeterostructuresSlide53
THANKS!
感谢您的关注Slide54
Can disorder enhance superconductivity? Anderson theorem is all but a theorem
Be careful with BCS+PerturbationAnderson theoremAnderson, J. Phys. Chem. Solids 11, 26 (1959
)
Gor'kov and
Abrikosov
Weak localization
Maekawa S, Fukuyama H, 1982
Finkelstein A M, 1987
Numerics
Trivedi
, Meir…..
S
trong coupling and disorder
Experiments
Pratap
, Sacepe…..
Strong disorder and no weak coupling
Abeles,… 60’s
AGG,Tezuka, 2011Slide55
Many body
Efimov Physics
Efimov
70’s
Bound states
Scaling Slide56
RGM
Born-OppenheimerSlide57
Strongly coupled field theory in d
N=4 Super-Yang MillsCFTAnti de Sitter spaceAdSWeakly coupled gravity in d+1
AdS
/CFT
Maldacena1997
Easy to compute in the gravity dual
Detailed dictionary
&
QCD Quark gluon plasma
Holographic superconductivity
2003
2008
2012
Quantum criticality, non-equilibrium.. Slide58Slide59Slide60Slide61Slide62
Multifractal eigenstates
Anderson Metal-Insulator Transitions
Wegner, Aoki,
Castellani
,
EfetovSlide63
Experimental testsSTM in thin films log2
distribution Transport to test higher global TcL ~ 5-10nm?DisorderNano engineering
Enhancement?
Only in boring materials?
MgB2?
FeSe
? Sure
Conclusion